Delete a Group Contact
You can delete a group contact as follows:
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Click the Recipients tab. See the following image:

The My Groups page appears.
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Search and locate the group to add the contacts in the My Groups tab. Organization admins can add contacts to the groups on the All Groups tab.
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Click the group name and open it. Otherwise, click Edit Group from the vertical ellipsis. See the following image:

The Group Settings page opens.
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Click Contacts under the Group Members section on the left navigation panel. See the following image:

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Search and locate the contact profile you want to edit. You can search using the name, mail ID or any custom attribute.
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Click the vertical ellipsis corresponding to the contact.
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Click Remove to delete a contact. The following image highlights the delete option:

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Click Yes to confirm the deletion.